Distribution of 40K, 238U, 232Th and Associated Radiological Risk in Quarry Soil of Chibok LGA, Borno State, Nigeria

Authors

  • Dominic Jauro
    University of Maiduguri
  • Musa Momoh
    Usmanu Danfodiyo University Sokoto
  • Yusuf Musa Ahijjo
    Usmanu Danfodiyo University
  • Lawal Sa'adu
    Federal University Gusau image/svg+xml

Keywords:

Gamma spectrometry, Quarry soil, Radiological Hazard, Cancer

Abstract

Effective monitoring of environmental radioactivity is essential for mitigating radiation-induced health risks such as cancer. In this study, the activity concentrations of 238U, 232Th, and 40K were measured in soil samples collected from thirteen sample points across chibok local government area. Gamma-ray spectrometry was employed for the analysis conducted at the center for energy research and development, Obafemi Awolowo university Ile-Ife. Osun state. The results, obtained indicate average activity concentrations of approximately 14.56 Bqkg-1 for 238U, 2.73 Bqkg-1 for 232Th, and 563.58 Bqkg-1 for 40K, with 40K being the dominant contributor to the overall specific activity. Furthermore, radiological parameters were evaluated, with the Absorbed dose rate (DAbs), Annual Effective Dose (AEDE), Radium equivalent (Raeq), External hazard index (Hex), Internal hazard index (Hin), Gamma activity index (Iγr), and Excess lifetime cancer risk (ELCR). Were all determined to assess the radiation hazard of the quarry soil yielding average values of 31.87 nGyh-1, 0.0391 mSvy-1, 61.855 Bq/kg, 0.167, 0.206, 0.506, and 0.00014 respectively, the result was also compared with other study as indicate in table 1. The current radiological concentration of the soil does not pose an immediate threat to human health or the environment. However, prolonged exposure over a lifetime could result to health risks for both workers and the general public, particularly for those in close proximity to the quarry. These findings underscore the importance of continuous radioactivity monitoring to protect both human health and other components of the locality.

Author Biographies

Dominic Jauro

Department of Physics

Musa Momoh

Department of Physics

Yusuf Musa Ahijjo

Usmanu Danfodiyo University Sokoto

Lawal Sa'adu

Department of Physics

Dimensions

Abai, I., Kamgba, F., & Ushie, P. (2021). Radiological Health Implications of Radiation Levels in Rock Fragments from Quarry Sites in Akamkpa, South-South Nigeria. Journal of Applied Physics, 13(6), 04 – 09. DOI: 10.9790/4861-1306020409

Abba, H. T., Waida, J., & Abdulsemiu, B. K. (2023). Annual Effective Dose Due to Background Gamma Radiation in Buni Gari, Yobe State. Communication in Physical Sciences, 10(I). http://gssrr.org/index.php?journal=JournalOfBasicAndApplied

Abdullahi, I. M. Yelwa, N. A. Abdulmumin, A. and Nabage, N. A. (2016). Groundwater Exploration in the Basement Complex Around Chibok Area in Northeastern Nigeria Using Vertical Electrical Sounding Method. Nigerian Journal of Basic and Applied Science 24 (2): 37- 44.

Abdullahi, Z. B., Dan Mallam, I. M., Ahijjo, Y. M., Maidamma, B., & Umar, M. (2025). Assessment of Radioactivity and Soil Dose Rate in Some Selected Areas of Wurno Mines-Nigeria. BIMA Journal of Science and Technology (2536-6041), 8(4b), 203-211. DOI: 10.56892/bima. v8i4B.1197 DOI: http://dx.doi.org/10.4314/njbas.v24i2.6

Aborisade, M. A., Gbadebo, A. M., Adedeji, O. H., Okeyode, I. C., & Ajayi, O. A. (2018). Excess lifetime Cancer risk and Radiation Pollution hazard indices in rocks and soil of some selected mining sites in Nasarawa State, Nigeria. Aegean Journal of Environmental Sciences, 3(3), 1-18.

Agbalagba, E. O., Chaanda, M. S., & Egarievwe, S. U. (2021). Assessment of solid mineral to soil radioactivity contamination index in selected mining sites and their radiological risk indices to the public. International Journal of Environmental Analytical Chemistry, 103(17), 5539-5557 DOI: https://doi.org/10.21203/rs.3.rs-496856/v1

Ahijjo, Y. M. Baba-Kutigi, A. N. Momoh, M. Bayawa, A. M. & Hussain, M. (2018). Radioactivity Concentrations in Soil Samples from Kandam, Gyalgyal, Burmawan masaka, Dinbisu and Giyawa Mines in Wurno LGA, Sokoto State, Nigeria. Asian Journal of Research and Reviews in Physics. 1 (4): 1 – 9. DOI: 10.9734/AJR2P/2018/45083

Ahijjo, Y. M., & Baba-Kutigi, A. N. (2023). Natural Radioactivity Levels and Radiological Hazards Indices of Soil Samples from Selected Mining Sites, Dange-Shuni, Sokoto State, Nigeria. Fudma journal of sciences, 7(1), 290-296. DOI: https://doi.org/10.33003/fjs-2023-0701-2065

Amodu. F. R., Ben. F., A. T. Agbele., B. N. Ben‑Festus., & O. A. Oyebanjo., (2024). Assessment of radionuclide concentration and associated risks in soils from Iperindo mining sites, Nigeria. Nature Discover Environment (2024) 2:17 https://doi.org/10.1007/s44274-024-00036-2

Belyaeva, O., Pyuskyulyan, K., Movsisyan, N., Saghatelyan, A., & Carvalho, F. P. (2019). Natural radioactivity in urban soils of mining centers in Armenia: dose rate and risk assessment. Chemosphere, 225, 859-870.

Ebibuloami, B. P., Ayorinde, O., Oluwagbenga, A. J., Kugbere, E., Adeola, O. M., & Olalekan, M. A. (2021). Detection efficiency of a NaI (Tl) gamma spectrometry system for measurement of low-level radioactivity. Physics Access, 1(01), 61-5. https://doi.org/10.47514/phyaccess.2021.1.1.010

Echeweozo, E. O., & Ugbede, F. O. (2020). Assessment of background ionizing radiation dose levels in quarry sites located in Ebonyi State, Nigeria. Journal of Applied Sciences and Environmental Management, 24(10), 1821-1826. DOI: https://dx.doi.org/10.4314/jasem.v24i10.17

Galadima, O. O., Orji, C. E., Rilwan, U., Ojike, P. E., & Omita, E. (2022). Assessment of the Effects of Radiation Exposure to Human Sensitive Organs Due to Quarry Mining in Kokona, Nasarawa and Toto of Nasarawa State Nigeria. Journal of Radiation and Nuclear Applications, An International Journal, 7, 29-38. http://dx.doi.org/10.18576/jrna/070204

Guagliardi, I., Zuzolo, D., Albanese, S., Lima, A., Cerino, P., Pizzolante, A., ... & Cicchella, D. (2020). Uranium, thorium and potassium insights on Campania region (Italy) soils: Sources patterns based on compositional data analysis and fractal model. Journal of Geochemical Exploration, 212, 106508. https://doi.org/10.1016/j.gexplo.2020.106508

Habu. T. Abba, and Yusuf M. Auwal, (2020). Radiation Impact Assessment of Quarrying Activities. A Case Study of Buni Gari Town, Yobe State, Nigeria. Dutse Journal of Pure and Applied Sciences (DUJOPAS), Vol. 6 No. 2.

ICRP, 2007. The 2007 Recommendations of the International Commission on Radiological Protection: Annals of the ICRP Publication 103. Elsevier, pp. 2–4.

Idris, S. B., Ibrahim, Y., & Abubakar, B. S. (2023). Radionuclide Analysis in the Soil Samples Collected Around Maiganga Coal Mining Site, Northeast, Nigeria, Using Gamma Ray Spectrometry. Gombe State Polytechnic Bajjoga, Journal of Science and Technology, 1(1), 40-47. https://www.jost.gspb.edu.ng

Jauro, D., Ngari, A. Z., Teru, P. B., & Yaram, A. T. (2024). Radon-222 Concentration and Health Implication in Borehole Water of Ngumari Costain, Jere, Local Government, Borno State. Nigerian Journal of Physics, 33(3), 134-141. https://doi.org/10.62292/njp.v33i3.2024.280

Jegede, O. A., Olaoye, M. A., Olagbaju, P. O., Makinde, V., & Badawy, W. M. (2023). Radiation risk assessment of quarry pit soil as construction material in Abeokuta, Nigeria: implications for environmental and public health. Isotopes in Environmental and Health Studies, 60(1), 90-102. https://doi.org/10.1080/10256016.2023.2285002

Joseph, S. R., Lumbi, L. W., Ibrahim, U., Yusuf, S. D., Mundi, A. A., Mustapha, I., ... & Oduh, I. O. (2022). Estimation of public radiological dose from mining activities in some selected cities in Nigeria. Dutse Journal of Pure and Applied Sciences, 8(1a), 22-35 https://dx.doi.org/10.4314/dujopas.v8i1a.3

Kareemah, A. L., Faiza, A., Nasir, N. A., Yakubu, A., & Fatima, K. (2024). Assessment of Radiation Dose Associated with Background Radionuclides in Quarry Soil at Dawakin-Kudu LGA Kano, Nigeria. Nigerian Journal of Physics, 33(1), 126-137.

Karuppasamy, M. B., Natesan, U., Seethapathy, C., & Seshachalam, S. (2024). Environmental radioactivity, radiological hazards, and trace elements assessment of nearshore sediment in the Bay of Bengal. International Journal of Sediment Research, 39(1), 70-82.

Khaleed, S. K., Joseph, E., & Ubaidullah, A. (2024). Natural Radioactivity and Environmental Risk Assessment of Rock Samples at Gidan Tagwaye Granite Quarry Site in Dutse. Area of Jigawa State using Gamma-Ray Spectrometry European Journal of Science, Innovation, www.ejsit-journal.com

Manisa, K., Erdogan, M., Usluer, A., Cetinkaya, H., Isik, U., Sahin, L., & Zedef, V. (2021). Assessment of natural radioactivity level of soil and water in the region of Çorlu (Turkey). Journal of Radioanalytical and Nuclear Chemistry, 329(3), 1213-1221. https://doi.org/10.1007/s10967-021-07906-6

Muhammad, A., & Abbasi, A. (2025). Determination of natural radioactivity concentrations and risk assessment in soil from mining sites in Minna environs, Niger State, Nigeria. Journal of Radioanalytical and Nuclear Chemistry, 1-9.

Nduka, J. K., Umeh, T. C., Kelle, H. I., Ozoagu, P. C., & Okafor, P. C. (2022). Health risk assessment of radiation dose of background radionuclides in quarry soil and uptake by plants in Ezillo-Ishiagu in Ebonyi South-Eastern Nigeria. Case Studies in Chemical and Environmental Engineering, 6, 10026 https://doi.org/10.1016/j.cscee.2022.100269

Obasi, I. A., Ogwah, C., Selemo, A. O. I., Afiukwa, J. N., & Chukwu, C. G. (2020). In situ measurement of radionuclide concentrations (238 U, 40 K, 232 Th) in middle Cretaceous rocks in Abakaliki–Ishiagu areas, southeastern Nigeria. Arabian Journal of Geosciences, 13, 1-9 https://doi.org/10.1007/s12517-020-05360-4

Ofomola, O. M., Ugbede, F. O., & Anomohanran, O. (2023). Environmental risk assessment of background radiation, natural radioactivity and toxic elements in rocks and soils of Nkalagu quarry, Southeastern Nigeria. Journal of Hazardous Materials Advances, 10, 100288.

Ohakwere-Eze, M. C., Nafiu, M., Singh, S. K., Kabiru, M., & Simon, J. (2024). Assessment of Natural Radioactivity and Radiation Hazard in Soil and Rock Samples from Mining Sites within North-Eastern Nigeria. Physics Access, 4(2), 74-84.

Olanya. A, Okellob. D, Oruru. B, Kisolo. A, (2022). The Primordial Radionuclides Activity Concentrations and Associated Minerals in Rocks from Selected Quarries in Northern Uganda. International Journal of Sciences: Basic and Applied Research (IJSBAR), 66(1), pp 45-65

Omonokhua, M., Ayomanor, B., & Dawuk, D. (2022). Evalaution of Backgroud Ionising Radiation Levels and Excess Lifetime Cancer Risk in a Quarry Site in Tamma: Ionising Radiation Levels and Excess Lifetime Cancer Risk in a Quarry Site. Nasara Journal of Science and Technology, 9(1), 1-7.

Onudibia, M. E., Da Silva, P. S. C., Essiett, A. A., Zahn, G. S., Genezini, F. A., Imeh, E. E., & Okoh, F. O. (2023). Examination of Natural Radioactivity Concentration and Radiological Exposure of Soil Within Mining Site in Umuahia South Abia State Nigeria, Using High Purity Germanium (HPGe) Gamma Ray Spectrometry http://dx.doi.org/10.18576/jrna/080304

Sospeter, G., Paul, N., & Francis, N. (2024). Naturally occurring radioactive materials and their activity levels in “machine-cut stone” quarries in Juja Sub County, Kiambu County, Kenya. Journal of Agriculture, Science and Technology, 23(2), 11-24. https://doi.org/10.4314/jagst.v23i2.2

Ugbede, O. F. (2020). Distribution of 40K 238U and 232Th and Associated Radiological Risk in River Sand Sediments Across Enugu East, Nigeria. Journals of Environmental Nanotechnology, Monitoring and Management, (Elervier).14 (100317). https://doi.org/10.1016/j.enmm.2020.100317

UNSCEAR (2000). Sources and Effects of Ionizing Radiation. United Nations Scientific Committee on the Effects of Atomic Radiation. United Nations, New York.

Vesna, M. Goran, M. Milos, S. Branko, R. Dragana, K. & Dragoslav, N (2021). A preliminary survey of natural radionuclides in soil and indoor radon in the town of Nis, Serbia Journal of Radioanalytical and Nuclear Chemistry (Springer), 329: 671 – 677. https://doi.org/10.1007/s10967-021-07851-4

World Health Organisation (WHO). (2008). Report on Radiation and Health

World Health Organisation (WHO). (2022). Report on Radiation and Health

Yadav, J., Khyalia, B., Kumar, N., Panghal, A., Singh, P. P., Devi, S., & Dalal, R. (2024). Assessment of natural radioactivity in soil and water in the upper Himalayas region along the Manali–Leh highway, India. Journal of Radioanalytical and Nuclear Chemistry, 333(6), 3075-3086. https://doi.org/10.15415/jnp.2021.82018

Published

2025-09-22

How to Cite

Jauro, D., Momoh, M., Ahijjo, Y. M., & Sa'adu, L. (2025). Distribution of 40K, 238U, 232Th and Associated Radiological Risk in Quarry Soil of Chibok LGA, Borno State, Nigeria. Nigerian Journal of Physics, 34(3), 117-124. https://doi.org/10.62292/10.62292/njp.v34i3.2025.420

How to Cite

Jauro, D., Momoh, M., Ahijjo, Y. M., & Sa'adu, L. (2025). Distribution of 40K, 238U, 232Th and Associated Radiological Risk in Quarry Soil of Chibok LGA, Borno State, Nigeria. Nigerian Journal of Physics, 34(3), 117-124. https://doi.org/10.62292/10.62292/njp.v34i3.2025.420

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